To add to what the others have mentioned, you can consider using a 3.66” stroke crank out of a 368 Lincoln. Rod and main bearing sizes are the same so that part is doable. Not sure if the timing sets are compatible though. That would be a 0.160" stroke increase if it's a drop in. Increasing the cubic inch displacement is the easiest way to up the horsepower and in the case of more stroke, gobs more lowend torque. If you’re buying custom pistons, then the cost doesn’t change for putting the wrist pin in a different spot to accommodate more stroke.
Although you mentioned that that you were not interested in offset grinding the crankshaft, the LYB engines do appear to be open to much more stroke than was available from the factory. The cam to crank centerline is actually 0.100” more on the LYB engines than the FE engines which means the potential for up to and potentially more than 4.25” stroke is there if you want to get creative on offset grinding the LYB crank to a smaller journal for additional stroke. This will of course require a different connecting rod.
On the camshaft, try to get one with a short lobe centerline (ie. 106° or 108°) as the LYB engines respond nicely to these. The valve placement in the heads being so far apart helps to explain in part why the LYB engines favor a smaller lobe centerline.

Lorena, Texas (South of Waco)